Error: number of observations (=337) <= number of random effects (=344) for term (1 + Predictor 2 | Grouping variable); the random-effects parameters and the residual variance (or scale parameter) are probably unidentifiable

General
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2

It would help if you could post your code as a reprex and include your data (or at least enough of it to demonstrate the problem), either in the reprex or using the dput() function from base R.